【药物名称】Alemcinal, ABT-229, A-81229
化学结构式(Chemical Structure):
参考文献No.21494
标题:4''-Deoxyerythromycin derivs.
作者:Lartey, P.A.; Nellans, H.N.; Klein, L.L.; Faghih, R. (Abbott Laboratories Inc.)
来源:EP 0623021; JP 1994511257; US 5578579; WO 9313780
合成路线图解说明:

The selective acetylation of erythromycin B (I) with acetic anhydride in methylene chloride gives the 2'-O-acetyl derivative (II), which is treated with thiocarbonyldiimidazole (CSDI) and DMAP in dichloromethane to yield the 4''-O-thiocarbonyl derivative (III). The reduction of (III) with Bu3SnH in refluxing toluene affords 2'-O-acetyl-4''-deoxyerythromycin B (IV), which is deacetylated in refluxing methanol giving 4''-deoxyerythromycin B (V). The reaction of (V) with AcOH and NaHCO3 yields the hemiketal (VI), which is demethylated at the NMe2 group by means of I2, NaOAc and Na2S2O3 affording the methylamino compound (VII). Finally, this compound is submitted to a reductive alkylation with acetaldehyde (VII) and H2 over Pd/C in methanol.

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