【药物名称】
化学结构式(Chemical Structure):
参考文献No.547136
标题:(R)-3,3,3-trifluoro-2-hydroxy-2-methyl-propionamides are orally active inhibitors of pyruvate dehydrogenase kinase
作者:Aicher, T.D.; Anderson, R.C.; Bebernitz, G.R.; Coppola, G.M.; Jewell, C.F.; Knorr, D.C.; Liu, C.; Sperbeck, D.M.; Brand, L.J.; Strohschein, R.J.; Gao, J.; Vinluan, C.C.; Shetty, S.S.; Dragland, C.; Kaplan, E.L.; DelGrande, D.; Islam, A.; Liu, X.; et al.
来源:J Med Chem 1999,42(15),2741
合成路线图解说明:

Alkylation of an equimolecular mixture of trans-2,5-dimethylpiperazine dihydrochloride (I) and the free base (II) with benzyl chloride produced the racemic monobenzyl piperazine, which was resolved using (-)-tartaric acid to yield the required (2R,5S)-isomer (III). (R)-3,3,3-Trifluoro-2-hydroxy-2-methylpropionic acid (IV) was protected as the silyl derivative (V) using bis(trimethylsilyl)urea, and subsequently converted to acid chloride (VI) by means of oxalyl chloride. Coupling of acid chloride (VI) with the chiral piperazine (III) afforded amide (VII), which was desilylated in methanolic HCl yielding (VIII). Hydrogenolysis of the N-benzyl group of (VIII) over Pd/C gave piperazine (IX). Finally, coupling of (IX) with 4-cyanobenzoyl chloride (X) furnished the corresponding bisamide.

Drug Information Express,Drug R&D,Chemical Database,Patent Search.
Copyright © 2006-2024 Drug Future. All rights reserved.Contact Us